Loki is confirmed, and has already been cast: Tom Hiddleston.
_V_'s post implies that there's going to be another villain, to be played by Colm Feore.
If they weren't going for younger actors, I think he would absolutely be a great Loki. But that was announced months ago...I'm rather intrigued who he'll be playing because, like you said, Thor doesn't really have a typical assortment of villains.
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"There is always some madness in love. But there is also always some reason in madness." - Friedrich Nietzsche
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