Max Zorin, absolutely.
Christopher Lee's Francisco Scaramanga was pretty good too.
Pleasance's take on Blofeld in You Only Live Twice was a big high point of the movie. Although, I hated how Charles Gray made Blofeld look like a complete wussy in Diamonds Are Forever.
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"If you gaze for long into an abyss, the abyss gazes also into you." - Friedrich Nietzsche
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