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I'd recommend FLCL. Really bizarre, cool, transgressive anime. Cronenberg's Existenz has moments of intense surrealism. Vampyr is definitely on target on that list, and so is Videodrome. If you haven't seen Videodrome, by all means get ahold of it. For surreal atmosphere, I would say the Wicker Man is a triumph. Television wise, I'd say the biggest triumphs of surrealism are Twin Peaks and the Prisoner. See the Prisoner.
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